Figueres: Visit the Dali museum (we did not do it but everyone tells us we missed out on one of the best museums).
Have some tapas and some beers at El Dynamic Cerveseria.
Girona: Good for a city trip or a side trip if you are visiting Barcelona. Trains between Barcelona Sants and Girona takes you abt 1H20min. Have lunch at La Fabrica Girona and go for a coffee to Espresso Mafia (see WeLike).